Growing Interest in Carbon Nanotube

The report of Kroto et al. in 1985 on the discovery of "bulkyball", fullerene C60 molecule led into a new beginning in carbon materials and a huge interest in their sciences. Sumio Iijima of NEC Laboratory in Tsukuba observed MWNTs with high-resolution transmission electron microscopy (TEM) in 1991, and two years later he observed SWNTs. While for the first time, researchers at the William Rice University synthesised bundles of SWNTs in 1996, and most recently, in 2003 Fakhru'l-Razi, Iyuke and co-workers synthesised SWNTs intertwined bundles that are similar to the ship anchor rope shown in Fig. 10.2. This trend had originated opportunities for quantitative experimentations on carbon nanotube science. As soon as 2000, the growing interest in nanotubes has resulted in overwhelming out pour of publications and patents as compared to other nanomaterials. A relatively comprehensive survey by Gupta and Dwivedy has presented internationally patenting activities from 1987 to 2001 with 226 inventions drawn from the United States (56%), Japan (28%), South Korea (9%) and the remainder from other countries to reveal the current trend of interest in developing carbon nanotube technology towards commercialisation. Table 10.1 presents selected inventions of carbon nanotube science and technology. The growing interest in carbon nanotubes has currently attracted a vast volume of literature, while the coverage in R&D and discussions in general indicate great promises into the future. This is due to the fact that carbon nanotubes possess tremendous potentials for applications as a result of their unique properties in thermal and electrical conductivities, high strengths and stiffness, etc. These properties are directly connected to the carbon atom as the building block, which in turn is so unique among the elements in its ability to exist in a wide variety of structures and forms.

Table 10.1 Selected inventions in carbon nanotubes research in chronological order (Gupta and Dwivedy 2004)

Invention

Reference

Carbon fibrils, method for producing same 34

and compositions containing same

Carbon fibrils and method for producing same 23

Uncapped and thinned carbon nanotubes and 23

process

Carbon nanotubule enclosing a foreign 21

material

Process of isolation of carbon nanotubes from 14 a mixture containing carbon nanotubes and graphite particles

Method and device for the production of 13

carbon nanotubes

Process for the separation of carbon nanotubes 11 from graphite

Storage of hydrogen in layered nanostructures 23 Process for separating components from 24

gaseous streams

Method of purifying carbon nanotubes 13

Process for purifying uncapping and 19

chemically modifying carbon nanotubes

Method for producing encapsulated 12

nanoparticles and carbon nanotubes using catalytic disproportionation of carbon monoxide

Method of forming carbon nanotubes on a 16

carbonacous body, composite material obtained thereby and electron beam source element using same

Method for making carbon nanotubes 12

Field emission device having nanostructured 39 emitters

Graphitic nanotubes in luminescence assays 8

Nanometer-scale microscopy probes 9

Field emission cold-cathode device 27

Field emission electron source 20

Method for manufacturing carbon nanotubes 17 as functional elements of MEMS devices Method of making ropes of single walled 9 carbon nanotubes

Electron-emitting source and method of 13 manufacturing the same

Process for fabricating article comprising 9 aligned truncated carbon nanotubes Article comprising enhanced nanotube emitter 13 structure and process for fabricating article_

Tennet et al. 1987 Tennet et al. 1992 Green and Tsang 1994

Ajayan et al. 1993 Uchida et al. 1994

Ohshima et. al. 1996

Ikazaki et al. 1997 Rodriguez et al. 1997 Rodriguez et al. 1997 Ebbesen et al. 1997 Hiura and Ebbesen 1997

Nolan et al. 1998

Yamamoto et. al. 1998

Olk, 1998

Debe, 1998

Massey et al. 1999 Lieber et. al. 2000 Nakamoto, 2000 Zettl and Cohen 2000

Mancevski, 2000 Smalley et al. 2001 Uemura et al. 2001 Jin et al., 1999 Jin et al. 2001

Fig. 10.2. Typical SWNTs intertwined into bundles of ropes (Fakhru'l et al. 2003)
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